In hydrology, the relationship between water storage and flow is still fundamental in characterizing and modeling hydrological systems. However, this simplification neglects important aspects of the variability of the hydrological system, such as stable or instable states, tipping points, connectivity, etc. and influences the predictability of hydrological systems, both for extreme events as well as long-term changes. We still lack appropriate data to develop theory linking internal pattern dynamics and integral responses and therefore to identify functionally similar hydrological areas and link this to structural features. We plan to investigate the similarities and differences of the dynamic patterns of state variables and the integral response in replicas of distinct landscape units. A strategic and systematic monitoring network is planned in this project, which contributes the essential dynamic datasets to the research group to characterize EFUs and DFUs and thus significantly improving the usual approach of subdividing the landscape into static entities such as the traditional HRUs. The planned monitoring network is unique and highly innovative in its linkage of surface and subsurface observations and its spatial and temporal resolution and the centerpiece of CAOS.
The formation of biogeochemical interfaces in soils is controlled, among other factors, by the type of particle surfaces present and the assemblage of organic matter and mineral particles. Therefore, the formation and maturation of interfaces is studied with artificial soils which are produced in long-term biogeochemical laboratory incubation experiments (3, 6, 12, 18 months. Clay minerals, iron oxides and charcoal are used as major model components controlling the formation of interfaces because they exhibit high surface area and microporosity. Soil interface characteristics have been analyzed by several groups involved in the priority program for formation of organo-mineral interfaces, sorptive and thermal interface properties, microbial community structure and function. Already after 6 months of incubation, the artificial soils exhibited different properties in relation to their composition. A unique dataset evolves on the development and the dynamics of interfaces in soil in the different projects contributing to this experiment. An integrated analysis based on a conceptual model and multivariate statistics will help to understand overall processes leading to the biogeochemical properties of interfaces in soil, that are the basis for their functions in ecosystems. Therefore, we propose to establish an integrative project for the evaluation of data obtained and for publication of synergistic work, which will bring the results to a higher level of understanding.
Although global pesticide use increases steadily, our field-data based knowledge regarding exposure of non-target ecosystems is very restricted. Consequently, this meta-analysis will for the first time evaluate the worldwide available peer-reviewed information on agricultural insecticide concentrations in surface water or sediment and test the following two hypotheses: I) Insecticide concentrations in the field largely exceed regulatory threshold levels and II) Additional factors important for threshold level exceedances can be quantified using retrospective meta-analysis. A feasibility study using a restricted dataset (n = 377) suggested the significance of the expected results, i.e. an threshold level exceedance rate of more than 50Prozent of the detected concentrations. Subsequent to a comprehensive database search in the peer-reviewed literature of the past 60 years, analysis of covariance with the relevant threshold level exceedance as the continuous dependent variable (about 10,000 cases) will be performed and the impact of significant predictor variables will be quantified. Parameters not yet considered in pesticide exposure assessment will be included as independent variables, such as compound class, environmental regulatory quality, and sampling design. The simultaneous presence of several insecticide compounds as a well as their metabolites will also be considered in the evaluation. The present approach may provide an innovative and integrated view on the potential environmental side effects of global high-intensity agriculture and in particular of pesticides use.
Current and future global warming will cause the degradation of mountain permafrost, which may strongly influence the stability of permafrost slopes or rock walls with potentially hazardous consequences. Due to the strong heterogeneity of both the thermal regime and the ground composition of mountain permafrost, its response to atmospheric forcing can however be highly variable for different landforms and within short distances. The spatial distribution of ice and liquid water is important for determining the sensitivity of a specific permafrost occurrence to climate change because of their large influence on the pace of temperature changes (by effects of latent heat) and their importance for geotechnical properties of the ground. Detailed knowledge of the material properties and internal structures of frozen ground is therefore an important prerequisite to determine the sensitivity of permafrost to climate change. Except for the active layer ice and water contents and their temporal and spatial variability usually cannot be measured directly. Geophysical methods are sensitive for the ice and liquid water content in the ground. With the proposed collaboration, two similar but complementary approaches to quantify the composition of the ground based on 2D sections of geophysical data will be combined for an improved determination of ice and water contents in permafrost regions. The so-called 4-phase model (4PM) is based on two simple petrophysical relationships for electrical resistivity and seismic velocity and estimates volumetric fractions of ice, water, and air within the pore volume of a rock matrix by jointly using complementary data sets from electric and seismic measurements. Due to inherent ambiguities in the model it is still restricted to specific cases and often allows only a rough estimation of the phase fractions. Major drawbacks of the current 4PM comprise the unsatisfactory discrimination between rock and ice and its under-determinedness, requiring the prescription of the porosity and further parameters. The so-called RSANN model (developed and used by the host institution) uses the technique of simulated annealing (a Monte-Carlo-type stochastic simulation approach) as an optimization tool for the integration of electrical resistivity and P-wave velocity to derive 2D sections of porosity, water saturation and volumetric water content. The simulated annealing technique allows - due to its iterative procedure - more parameters to be predicted instead of being prescribed as in the 4PM. The objective of the proposed collaboration is to combine the advantages of the two algorithms (4PM and RSANN) to overcome the shortcomings of the 4PM in order to improve the reliability of the determined ice and liquid water contents. (...)
Quality standards to assess the chemical status of water bodies under the Water Framework Directive are often based on a few standardized laboratory tests and fixed assessment factors for extrapolation to the field situation. If larger data sets including tests with non-standard species are available, a statistical extrapolation approach, the Species Sensitivity Distribution approach (SSD) is applied. For assessing the remaining uncertainty on the SSD, the threshold concentration derived can be compared with data from field monitoring or model ecosystem studies. Taking the priority substance Ni as an example we present the use of microcosms to test the protectiveness of the quality standard derived from laboratory toxicity tests. The study was conducted in 14 microcosms including a natural sediment layer and an overlaying water volume of 750 L located in a greenhouse. After a pre-treatment period for establishing a diverse aquatic community of phytoplankton, zooplankton, periphyton and snails, Ni solution was added to reach concentrations of 6, 12, 24, 48 and 96 micro g Ni/L in two microcosms each. Four microcosms served as untreated controls. To achieve the intended constant exposure over the test period of four months, Ni concentrations were frequently determined in the microcosms and appropriate amounts of nickel solution were added mostly on a daily basis. Parameters known to affect Ni toxicity, i.e. water hardness, pH, and dissolved organic carbon, were also measured. Population abundance and community structure were analysed for difference to the dynamics in the controls. In the microcosms with 48 and 96 micro g Ni/L long-term effects on phytoplankton, rotifers, snails and, due to reduced grazing by snails, indirectly on the periphyton biomass were observed. Only minor, and/or temporary deviations from controls, i.e., for single sampling dates, were found for a few algae taxa at lower concentrations. Because these deviations showed no clear dose-response and were not found at the end of the study they were not seen as adverse effects. However, for the snail (Lymnaea stagnalis), effects on the trend of population development could not be excluded at 24 micro g/L. Thus, the overall No Observed Effect Concentration (NOEC) for a chronic exposure to nickel in this microcosm study was considered to be 12 micro g Ni/L. This NOEC confirms the protectiveness of the quality standard derived from the laboratory single species tests.
The goal of the proposal is to explore the structure and functioning of metacommunities in ecological compensation areas at a multi-trophic level. First, we will assess the effect of plant diversity and herbivore and/or predator exclusion on metacommunity functioning in sown wildflower strips. We will document the communities inhabiting these experimental plots, paying attention at interactions between species, and with consideration of larger consumers linking these habitats with the surrounding matrix. Second, we will explore the relationship between various measures of the environment (isolation, habitat size) and descriptors of the metacommunities (diversity, composition, abundances, and productivity of various taxonomic groups, food-web structure, temporal variability, local invasions and extinctions). Third, using a high-quality dataset on quantitative food webs and the present data, we will conduct meta-analyses to test various models of community organisation (neutral models of biodiversity, species-area relationship in trophic levels, regional similarity hypothesis, food-web structure). Fourth, we will develop various models describing food-web structure and metacommunities dynamics. We will synthesize our results to develop a theory of 'meta food-webs'. Fifth, we will apply the gained knowledge to improve current agri-environment schemes. The study of species interactions in spatially structured metacommunities is comprehensive and global. As such, this project has a strong potential to provide fundamental insight into conservation biology. This project is multidisciplinary, putting together practitioners, ecologists and mathematicians, and is expected to yield important results both of fundamental and conservation relevance. We will use various methodologies to reach our goals. For the first part, we will set up an experiment with replicated sown wildflower strips where plant species richness and the abundance of major predators (foxes and birds of prey) and/or of major herbivores (voles and slugs) will be controlled (balanced incomplete block design). The other parts will rely on classical meta-analyses, multivariate statistics, and mathematical modelling. For the latter part, we will develop stochastic models to explore the dynamics of communities.
In contrast to their advances in other areas, weather forecast models have not been successful in improving the Quantitative Precipitation Forecast during the last 16 years. One reason for this stagnation is the lack of comprehensive, high-quality data sets usable for model validation as well as for data assimilation, thus leading to improved initial fields in numerical models. Theoretical analyses have identified the requirements measured data have to meet in order to close the gaps in process understanding. In field campaigns, it has been shown that the newest generation of remote sensing systems has the potential to yield data sets of the required quality. It is therefore time to combine the most powerful remote sensing instruments with proven ground-based and airborne measurement techniques in an Intensive Observations Period (IOP). Its goal is to serve as a backbone for the SPP 1167 by producing the demanded data sets of unachieved accuracy and resolution. This requires a sophisticated scientific preparation and a careful coordination between the efforts of the institutions involved. For the first time, the pre-convective environment, the formation of clouds and the onset and development of precipitation as well as its intensity will be observed in four dimensions simultaneously in a region of sufficient size. This shall be achieved by combining the IOP with international programs and by collaboration between leading scientists in Europe, US and other countries. Thus, the IOP is a unique opportunity to make Germany the setting of an international field campaign featuring the newest generation of measurement systems such as scanning radar and lidar and leading to outstanding advances in atmospheric sciences.
A GC-MS/GC-IRMS for the molecular-level analyses of organic matter and the isotopic characterization of inorganic and organic compounds in aquatic and terrestrial ecosystems Stable isotopes represent a valuable means to constrain specific biogeochemical processes in natural environments. The main objective of the project is to develop an Environmental Laboratory for Aquatic and Terrestrial Biogeochemistry, which will support research that will make use of molecular-level characterization and (compound-specific) isotope ratio determination methods to assess a wide spectrum of biogeochemical transformations in the natural environment and in the laboratory, and to study sources and the fate of organic compounds in marine, freshwater, and soil systems. One of the major goals of the projects that make use of the new instrumental capacities is to understand the interactions of the bio- with the geo- and atmosphere with respect to the transport of organic materials and the transformation of inorganic and organic compounds by plants and microorganisms, which is of ultimate importance for the reduction of green house gases and the cycling of elements in aquatic and terrestrial ecosystems. A prime objective will be to use stable isotope measurements to constrain specific biogeochemical and metabolic processes, as well as sources, transport and degradation of organic matter in aquatic and terrestrial environments, and, in turn, to use these constraints to obtain improved estimates on global and regional C and N fluxes, in modern environments as well as in the past. Planned research themes include: I) using lipid biomarker approaches to study microbial communities in various marine and freshwater environments, II) characterizing organic matter components in lacustrine sediments as well as in soils, and identifying the mechanisms responsible for the longer-term sequestration and degradation of organic C and the emission of greenhouse gases, III) understanding the metabolic pathways of C and N during the symbiosis between microorganisms and plants, and IV) generating data sets for the isotopic composition of nitrate and other N species in various aquatic systems in order to characterize the controls on isotope fractionation of specific N cycle reactions. The spectrum of investigated ecosystems will range from Swiss soil and groundwater systems and small lakes to hydrothermal vent systems in the deep ocean, and the spatial scale of the planned research extends from enzyme biogeochemistry to ocean-scale circulation.
AIR4EU addresses the needs for policy-orientated research on integrated air quality (AQ) assessment by monitoring methods and modelling at different temporal and spatial scales for regulated components in Europe: PM10 (and PM2.5), NO2, CO, SO2, O3 and benzene. Policy support on AQ assessment has been recognised a priority issue within the 'Clean Air for Europe-CAFE' programme. There are a wide variety of AQ assessment methods based upon monitoring and modelling, but these methods depend on the spatial and temporal scales, and are often not or only partially compatible. Consequently, there is a need for scientific sound and practical recommendations on how to integrate monitoring and modelling methods into internally consistent, comprehensive and cost-effective assessment methods. The aim of AIR4EU is to provide recommendations on AQ assessment for different temporal and spatial scales: ranging from hourly to annual and from 'hotspot'/street to continental scale. Case studies are implemented with partners in Paris, Berlin, Prague, London, Athens, Rotterdam and Oslo, to test and further develop the recommendations. AIR4EU will also prepare AQ maps at different scales in Europe based upon available data sets (monitoring, meteorology and emissions) and the recommended methods. The cooperation of European top-scientists from six member states representing four universities, two research institutes and eight user-partners will support the establishment of the European Research Area. AIR4EU will co-operate with on-going relevant projects (e.g. ENV-e-CITY; OSCAR; CLEAR; MERLIN) and networks (e.g. INTEGAIRE, CITY-Delta; POLIS), and specific liaison will be established with the CAFE programme. AIR4EU will disseminate its results by a Website and through Newsletters and Workshops to the scientific community, environmental authorities, policy makers and other stakeholders in AQ in Europe. Prime Contractor: Nederlandse Organisatie voor Toegepast Natuurwetenschappelijk Onderzoek - TNO; Delft; Netherlands.
Satellite measurements strongly contribute to the understanding of the processes related to stratospheric ozone loss, e.g. by global and long term monitoring of ozone and its depleting substances. For instance, measurements performed in limb geometry by SCIAMACHY on ENVISAT largely improved the knowledge about the vertical distribution of species like BrO and OClO only recently. However, there are still important open questions, like e.g. the chlorine activation processes on different kinds of aerosols and polar stratospheric clouds. Also, the role of very short lived species in the stratospheric bromine budget or the effects of a possible enhancement of the Brewer-Dobson circulation are not fully understood.Globally, the vertical distribution of ozone depleting species varies significantly in space and time due to solar illumination, atmospheric chemistry and transport. Especially strong gradients occur near the twilight zone or across stratospheric transport barriers (polar vortex boundary, subtropical transport barriers). These regions are of particular importance for chemistry and transport of the lower stratosphere and upper troposphere, since they separate air masses on large scales but also enable exchange between them.Standard 1-D profile retrievals, which assume horizontal homogeneity, result in large systematic biases due to neglecting the effect of horizontal gradients on the measurement. We propose to develop, improve and apply a tomographic profile retrieval algorithm, which optimally combines the information provided by the SCIAMACHY limb and nadir measurements. An improved global dataset of 3D stratospheric profiles for NO2, BrO and OClO for the 10 years of the SCIAMACHY mission (2002-2012) will be developed, compared to atmospheric chemistry simulations and applied to selected questions of atmospheric science. The dataset developed in this project will be very useful for investigating the complex interplay of stratospheric chemistry and transport processes, and will help to reduce the uncertainties in the distribution of ozone depleting species, in particular for regions with large horizontal inhomogeneity.
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