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METOP GOME-2 - Sulfur Dioxide (SO2) - Global

Gridded Level 3 SO2 total column densities derived from the Metop/GOME-2-instruments. Volcanoes are the largest soures of SO2 in the atmosphere, depending on the erruption the Sulfurous compounds can be injected into stratosphere but in most cases it stays within the troposphere. Another important source is the coal combustion. Desulfurisation facilities within the power stations have reduced the sulfur emissions around the globe. In the stratosphere sulfur is a key component for building up aerosols, which reflect parts of the solar irradiation. The total SO2 column is retrieved from GOME solar back-scattered measurements in the ultraviolet wavelength region [using the DOAS method]. Depending on the plume SO2 can be a very strong absorber, because of that the ODAS retrieval might have some smaller issues, they can be reduced by choosing different wavelenght ranges depending on the signal. We apply three different fitting windows between 310 and 360nm. For the AMF, we assume a plumeheight of 6 km altitude. The Global Ozone Monitoring Experiment-2 (GOME-2) instrument continues the long-term monitoring of atmospheric trace gas constituents started with GOME / ERS-2 and SCIAMACHY / Envisat. Three instruments operate on board EUMETSAT's Meteorological Operational satellites MetOp-A, -B, and -C, launched in 2006, 2012, and 2018, respectively. GOME-2 measures a range of atmospheric trace constituents, with the emphasis on global ozone distribution. Furthermore, cloud properties and intensities of ultraviolet radiation are retrieved. These data are crucial for monitoring the atmospheric composition and the detection of pollutants. DLR generates operational GOME-2 / MetOp products in the framework of EUMETSAT's Satellite Application Facility on Atmospheric Composition Monitoring (AC-SAF).

Untersuchungen des Tagesgangs verschiedener Spurengase mit Hilfe der solaren Absorptionsspektroskopie im infraroten Spektralbereich im tropischen Westpazifik (TROPAC)

Der Ozean im Westpazifik ist mit Temperaturen von ganzjährig 30°C der wärmste Ozean der Welt. Im tropischen Westpazifik ist die Lufttemperatur der Grenzschicht weltweit am höchsten und die Ozonkonzentration am niedrigsten. Aufgrund der allgemeinen Advektion der Luftmassen in der unteren und mittleren Troposphäre aus dem Osten durch die Walker-Zirkulation über den Pazifik befindet sich die Luft über dem tropischen Westpazifik für längere Zeit in einer sauberen, warmen und feuchten Umgebung. Der Abbau von reaktiven Sauerstoff- und Ozonvorläufern wie NOx findet daher länger als anderswo in den Tropen, was zu sehr niedrigen Ozonkonzentrationen führte. Dies erhöht die Lebensdauer von kurzlebigen biogenen und anthropogenen Spurengasen. Darüber hinaus begünstigen hohe Meeresoberflächentemperaturen eine starke Konvektion im tropischen Westpazifik, was zu niedrigen Ozonmischungsverhältnissen in den konvektiven Ausflussgebieten in der oberen Troposphäre führen kann. Der Warmpool im Westpazifik ist auch eine wichtige Quellregion für stratosphärische Luft. Daher fallen die Region, in der die Lebensdauer kurzlebiger Spurengase erhöht ist, und die Quellregion der stratosphärischen Luft zusammen. Somit bestimmt die Zusammensetzung der troposphärischen Atmosphäre in dieser Region in hohem Maße auch die globale stratosphärische Zusammensetzung.Ozon ist aufgrund von Rückkopplungsprozessen zwischen Temperatur, Dynamik und Ozon ein wichtiges Spurengas in der Klimaforschung. Da der Warmpool im Westpazifik die Hauptquellenregion für stratosphärische Luft ist, ist die Kenntnis von Ozon und anderen kurzlebigen Spurengasen auch wichtig, um den Transport von Spurengasen in die Stratosphäre zu verstehen.Ziel unseres Projektes ist die Messung des Tagesgangs von Ozon und anderen Spurengasen mit Hilfe der hochauflösenden solaren Absorptions-FTIR-Spektroskopie. Die Messungen liefern die Gesamtsäulendichten von bis zu 20 Spurengasen. Für einige Spurengase erlaubt die Analyse der Spektrallinienform die Ableitung der Konzentrationsprofile in bis zu etwa vier atmosphärischen Höhenschichten. Ergänzt werden die Beobachtungen durch Ozonballonsondierungen, kontinuierliche Messungen der UV-Strahlung, und Modellrechnungen mit einem Chemie-Transport-Modell. Die Messungen sind für den Zeitraum August bis Oktober 2022 geplant, die Auswertung und Interpretation von November 2022 bis Januar 2023.

Brackish water rewetting of a temperate coastal peatland in NE Germany: Effects on Biogeochemistry, Microorganisms and Greenhouse gas emissions

The rewetting of drained peatlands is a promising measure to mitigate carbon dioxide (CO2) emissions by preventing the further mineralization of the peat soil through aeration. While freshwater rewetted peatlands can be significant methane (CH4) sources in the short-term, in coastal ecosystems the input of sulfate-rich seawater could potentially mitigate these emissions. The purpose of the data collection was to examine whether the presence of sulfate, known as an alternative electron acceptor, can cause lower CH4 production and thus, emissions by favoring the growth of sulfate-reducers, which outcompete methanogens for substrate. We therefore investigated underlying variables such as the methane-cycling microbial community along with CH4 fluxes and set them in context with CO2 fluxes along a transect in a coastal peatland before and directly after rewetting. In this way, a conclusion about the short-term greenhouse gas mitigation potential of brackish water rewetting of coastal peatlands could be drawn. This data collection consists of six data sets, with direct comparisons before and after rewetting of CO2 and CH4 fluxes (Tab. 2) and associated microbial communities (Tab. 1) being the main data. Pore water geochemistry (Tab. 1 and 3) and surface water parameters (Tab. 4) were collected simultaneously to provide potential explanatory variables. The sampling of continuous water level (Tab. 5) within wells and atmospheric weather data (air and soil temperature, relative humidity, photosynthetic photon flux density; Tab. 6) from a weather station was done in addition. Measurements started in June/July/August 2019 after field installation was finalized and were conducted on the drained coastal fen "Polder Drammendorf" on the island of Rügen in North-East Germany. On 26th November 2019, the dike was opened and channeled in order to rewet the peatland with brackish water. Before, the dike separated the peatland from the adjacent bay "Kubitzer Bodden", which is part of a brackish lagoon system connected to the Baltic Sea. Therefore, the peatland was nearly completely flooded and now resembles a shallow lagoon with high fluctuating water levels. We measured along a humidity (pre-rewetting)/water level (post-rewetting) gradient (stations 0-8) towards and across the main North-South oriented drainage ditch, including four stations on the Eastern side of the ditch (1–4), two ditch stations (0, 5) and two stations (6, 7) on the Western side of the ditch. Station 8 was chosen as an additional station farther towards the adjacent bay on the Western side, but was only accessible before rewetting. CH4 and CO2 fluxes (stations 0-7) were calculated from online gas concentrations measurements using laser-based analyzers and manual closed chambers (Livingston, G. P., & Hutchinson, G. (1995). Enclosure-based measurement of trace gas exchange: Applications and sources of error. In P.A. Matson, & R.C. Harriss (Eds.). Biogenic trace gases: Measuring emissions from soil and water (pp. 14–51). Blackwell Science Ltd., Oxford, UK). Soil cores for microbial, dissolved gas concentrations and isotopic analysis were taken using a Russian type peat corer (De Vleeschouwer, F., Chambers, F. M., & Swindles, G. T. (2010). Coring and sub-sampling of peatlands for palaeoenvironmental research. Mires and Peat, 7, 1–10) before and after rewetting. Each time, we took duplicates at stations 1-8 for this rather labor-intensive process and divided the core into four depth sections: surface, 5–20, 20–40 and 40–50 cm. Subsamples for dissolved gases and stable carbon isotope analyses were taken with tip-cut syringes with a distinct volume of 3 ml (Omnifix, Braun, Bad Arolsen, Germany) and immediately placed into NaCl-saturated vials (20 ml, Agilent Technologies, 5182-0837, Santa Clara, USA) leaving no headspace and closed gas-tight using rubber stoppers and metal crimpers (both: diameter 20 mm, Glasgerätebau Ochs, Bovenden, Germany). Absolute abundances of specific functional target genes, including methane- and sulfate-cycling microorganisms, were measured with quantitative PCR (qPCR) after DNA was extracted (GeneMATRIX Soil DNA Purification Kit, Roboklon, Berlin, Germany) and quantified (Qubit 2.0 Fluorometer, ThermoFisher Scientific, Darmstadt, Germany). Surface and pore water parameters were measured in parallel to the gas measurements and soil coring for microbial analyses. Most surface water variables (pH, specific conductivity, salinity, nutrients, oxygen, sulfate and chloride concentrations, DOC/DIC) were measured in-situ using a multiparameter digital water quality meter or taken to the laboratory as water samples for further analysis. Likewise, pore water/soil variables (pH, specific conductivity, nutrients, metals, sulfate and chloride concentrations, CNS) were either measured in-situ or taken to the laboratory as soil samples. While surface water analysis was only conducted in the drainage ditch before rewetting, it was done along the entire transect after rewetting. In contrast, pore water/soil analysis was mostly conducted before rewetting and only repeated occasionally after rewetting where possible.

Sonderforschungsbereich Transregio 172 (SFB TRR): Arktische Verstärkung: Klimarelevante Atmosphären- und Oberflächenprozesse und Rückkopplungsmechanismen (AC)3, Teilprojekt C02: Wechselwirkungen von Schnee auf Meereis mit atmosphärischen Bestandteilen inklusive Ruß

Gleichzeitige Beobachtungen von atmosphärischem Ruß, und Rußpartikeln in Schnee- und Bodeneigenschaften sind selten. Daher wird dieses Teilprojekt Flugzeug- und bodengebundene Beobachtungen von Aerosolen und Rußkonzentrationen kombinieren, sowie optische Schneeeigenschaften und deren Rückkopplungsmechanismen in der arktischen Region untersuchen. In-situ Messungen von atmosphärischen Rußpartikeln (boden- und flugzeuggetragen) in Verbindung mit Rußpartikeln in Schneeproben und Fernerkundungsbeobachtungen von Schneeeigenschaften werden zusammengefügt.

Minderung von Lachgasemissionen aus gemüsebaulich genutzten Böden durch Optimierung des Nacherntemanagements

Zielsetzung: Distickstoffmonoxid (N2O), allgemein bekannt unter dem Trivialnamen Lachgas, zählt neben Kohlenstoffdioxid (CO2) und Methan (CH4) zu den Spurengasen in der Atmosphäre, die maßgeblich zu den anthropogen bedingten Klimaveränderungen beitragen. Eine Hauptquelle für das Lachgas stellen landwirtschaftlich und gartenbaulich genutzte Böden dar. Im Zuge der Applikation von stickstoffhaltigen organischen und mineralischen Düngern werden mikrobielle Umsetzungen forciert, die zur N2O-Bildung führen. In dem geplanten Projekt soll ein neuer Ansatz zur Reduktion von Lachgasemissionen im Freilandgemüsebau entwickelt werden. Nach der Einarbeitung von leicht zersetzbaren Ernterückständen wird Lachgas mit besonders hoher Rate aus Böden freigesetzt. Ziel ist es, diese unerwünschten N-Abflüsse durch eine Optimierung des Nacherntemanagements zu minimieren. Mögliche Ansatzpunkte hierfür liegen in der Anwendung von Nitrifikationsinhibitoren, der Einarbeitungstechnik und in dem Einarbeitungstermin der Ernterückstände. Die vorgesehenen Maßnahmen sollen gleichzeitig auch zu einer Verringerung weiterer Stickstoffverluste durch Denitrifikation und Auswaschung von Nitrat beitragen. Insgesamt wird das Ziel verfolgt, die Stickstoffeffizienz bei der Erzeugung von Gemüse im Freiland zu erhöhen und damit die ökologische und ökonomische Nachhaltigkeit der Anbauprozesse zu verbessern.

Sentinel-5P TROPOMI Surface Nitrogendioxide (NO2), Level 4 – Regional (Germany and neighboring countries)

The TROPOMI instrument onboard the Copernicus SENTINEL-5 Precursor satellite is a nadir-viewing, imaging spectrometer that provides global measurements of atmospheric properties and constituents on a daily basis. It is contributing to monitoring air quality and climate, providing critical information to services and decision makers. The instrument uses passive remote sensing techniques by measuring the top of atmosphere solar radiation reflected by and radiated from the earth and its atmosphere. The four spectrometers of TROPOMI cover the ultraviolet (UV), visible (VIS), Near Infra-Red (NIR) and Short Wavelength Infra-Red (SWIR) domains of the electromagnetic spectrum. The operational trace gas products generated at DLR on behave ESA are: Ozone (O3), Nitrogen Dioxide (NO2), Sulfur Dioxide (SO2), Formaldehyde (HCHO), Carbon Monoxide (CO) and Methane (CH4), together with clouds and aerosol properties. This product displays the Nitrogen Dioxide (NO2) near surface concentration for Germany and neighboring countries as derived from the POLYPHEMUS/DLR air quality model. Surface NO2 is mainly generated by anthropogenic sources, e.g. transport and industry. POLYPHEMUS/DLR is a state-of-the-art air quality model taking into consideration - meteorological conditions, - photochemistry, - anthropogenic and natural (biogenic) emissions, - TROPOMI NO2 observations for data assimilation. This Level 4 air quality product (surface NO2 at 15:00 UTC) is based on innovative algorithms, processors, data assimilation schemes and operational processing and dissemination chain developed in the framework of the INPULS project. The DLR project INPULS develops (a) innovative retrieval algorithms and processors for the generation of value-added products from the atmospheric Copernicus missions Sentinel-5 Precursor, Sentinel-4, and Sentinel-5, (b) cloud-based (re)processing systems, (c) improved data discovery and access technologies as well as server-side analytics for the users, and (d) data visualization services.

Sentinel-5P TROPOMI - Aerosol Optical Depth (AOD), Level 3 - Global

Aerosol optical depth (AOD) as derived from TROPOMI observations. AOD describes the attenuation of the transmitted radiant power by the absence of aerosols. Attenuation can be caused by absorption and/or scattering. AOD is the primary parameter to evaluate the impact of aerosols on weather and climate. Daily AOD observations are binned onto a regular latitude-longitude grid. The TROPOMI instrument onboard the Copernicus SENTINEL-5 Precursor satellite is a nadir-viewing, imaging spectrometer that provides global measurements of atmospheric properties and constituents on a daily basis. It is contributing to monitoring air quality and climate, providing critical information to services and decision makers. The instrument uses passive remote sensing techniques by measuring the top of atmosphere solar radiation reflected by and radiated from the earth and its atmosphere. The four spectrometers of TROPOMI cover the ultraviolet (UV), visible (VIS), Near Infra-Red (NIR) and Short Wavelength Infra-Red (SWIR) domains of the electromagnetic spectrum. The operational trace gas products generated at DLR on behave ESA are: Ozone (O3), Nitrogen Dioxide (NO2), Sulfur Dioxide (SO2), Formaldehyde (HCHO), Carbon Monoxide (CO) and Methane (CH4), together with clouds and aerosol properties. This product is created in the scope of the project INPULS. It develops (a) innovative retrieval algorithms and processors for the generation of value-added products from the atmospheric Copernicus missions Sentinel-5 Precursor, Sentinel-4, and Sentinel-5, (b) cloud-based (re)processing systems, (c) improved data discovery and access technologies as well as server-side analytics for the users, and (d) data visualization services.

Sentinel-5P TROPOMI – Cloud Optical Thickness (COT), Level 3 – Global

This product displays the Cloud Optical Thickness (COT) around the globe. Clouds play a crucial role in the Earth's climate system and have significant effects on trace gas retrievals. The cloud optical thickness is retrieved from the O2-A band using the ROCINN algorithm. The TROPOMI instrument aboard the SENTINEL-5P space craft is a nadir-viewing, imaging spectrometer covering wavelength bands between the ultraviolet and the shortwave infra-red. TROPOMI's purpose is to measure atmospheric properties and constituents. It is contributing to monitoring air quality and providing critical information to services and decision makers. The instrument uses passive remote sensing techniques by measuring the Top Of Atmosphere (TOA) solar radiation reflected by and radiated from the earth and its atmosphere. The four spectrometers of TROPOMI cover the ultraviolet (UV), visible (VIS), Near Infra-Red (NIR) and Short Wavelength Infra-Red (SWIR) domains of the electromagnetic spectrum, allowing operational retrieval of the following trace gas constituents: Ozone (O3), Nitrogen Dioxide (NO2), Sulfur Dioxide (SO2), Formaldehyde (HCHO), Carbon Monoxide (CO) and Methane (CH4). Within the INPULS project, innovative algorithms and processors for the generation of Level 3 and Level 4 products, improved data discovery and access technologies as well as server-side analytics for the users are developed.

Sentinel-5P TROPOMI – Cloud Fraction (CF), Level 3 – Global

Global Cloud Fraction (CF). Clouds play a crucial role in the Earth's climate system and have significant effects on trace gas retrievals. The radiometric cloud fraction is retrieved from the UV using the OCRA algorithm. Daily observations are binned onto a regular latitude-longitude grid. The TROPOMI instrument aboard the SENTINEL-5P space craft is a nadir-viewing, imaging spectrometer covering wavelength bands between the ultraviolet and the shortwave infra-red. TROPOMI's purpose is to measure atmospheric properties and constituents. It is contributing to monitoring air quality and providing critical information to services and decision makers. The instrument uses passive remote sensing techniques by measuring the Top Of Atmosphere (TOA) solar radiation reflected by and radiated from the earth and its atmosphere. The four spectrometers of TROPOMI cover the ultraviolet (UV), visible (VIS), Near Infra-Red (NIR) and Short Wavelength Infra-Red (SWIR) domains of the electromagnetic spectrum, allowing operational retrieval of the following trace gas constituents: Ozone (O3), Nitrogen Dioxide (NO2), Sulfur Dioxide (SO2), Formaldehyde (HCHO), Carbon Monoxide (CO) and Methane (CH4). Within the INPULS project, innovative algorithms and processors for the generation of Level 3 and Level 4 products, improved data discovery and access technologies as well as server-side analytics for the users are developed.

Sentinel-5P TROPOMI – Ozone (O3), Level 3 – Global

Ozone vertical column density in Dobson Units as derived from Sentinel-5P/TROPOMI observations. The stratospheric ozone layer protects the biosphere from harmful solar ultraviolet radiation. Ozone in troposphere can pose risks to the health of humans, animals, and vegetation. The TROPOMI instrument aboard the SENTINEL-5P space craft is a nadir-viewing, imaging spectrometer covering wavelength bands between the ultraviolet and the shortwave infra-red. TROPOMI's purpose is to measure atmospheric properties and constituents. It is contributing to monitoring air quality and providing critical information to services and decision makers. The instrument uses passive remote sensing techniques by measuring the Top Of Atmosphere (TOA) solar radiation reflected by and radiated from the earth and its atmosphere. The four spectrometers of TROPOMI cover the ultraviolet (UV), visible (VIS), Near Infra-Red (NIR) and Short Wavelength Infra-Red (SWIR) domains of the electromagnetic spectrum, allowing operational retrieval of the following trace gas constituents: Ozone (O3), Nitrogen Dioxide (NO2), Sulfur Dioxide (SO2), Formaldehyde (HCHO), Carbon Monoxide (CO) and Methane (CH4). Daily observations are binned onto a regular latitude-longitude grid. Within the INPULS project, innovative algorithms and processors for the generation of Level 3 and Level 4 products, improved data discovery and access technologies as well as server-side analytics for the users are developed.

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